93 research outputs found
Spin-photo-currents generated by femtosecond laser pulses in a ferrimagnetic GdFeCo/Pt bilayer
© 2017 Author(s). Using THz emission spectroscopy, we detect spin-photo-currents from a ferrimagnetic amorphous alloy GdFeCo to an adjacent Pt capping layer. The currents are generated upon excitation of a GdFeCo/Pt heterostructure with femtosecond laser pulses. It is found that the polarization of the spin-polarized current is determined by magnetic sublattice sensitivity rather than the total magnetization, allowing for spin-polarized current generation when the net magnetization is zero
Two-magnon bound state causes ultrafast thermally induced magnetisation switching.
There has been much interest recently in the discovery of thermally induced magnetisation switching using femtosecond laser excitation, where a ferrimagnetic system can be switched deterministically without an applied magnetic field. Experimental results suggest that the reversal occurs due to intrinsic material properties, but so far the microscopic mechanism responsible for reversal has not been identified. Using computational and analytic methods we show that the switching is caused by the excitation of two-magnon bound states, the properties of which are dependent on material factors. This discovery allows us to accurately predict the onset of switching and the identification of this mechanism will allow new classes of materials to be identified or designed for memory devices in the THz regime
Optical determination of the Néel vector in a CuMnAs thin-film antiferromagnet
Recent breakthroughs in electrical detection and manipulation of antiferromagnets have opened a new avenue in the research of non-volatile spintronic devices.1-10 Antiparallel spin sublattices in antiferromagnets, producing zero dipolar fields, lead to the insensitivity to magnetic field perturbations, multi-level stability, ultrafast spin dynamics and other favorable characteristics which may find utility in fields ranging from magnetic memories to optical signal processing. However, the absence of a net magnetic moment and the ultra-short magnetization dynamics timescales make antiferromagnets notoriously difficult to study by common magnetometers or magnetic resonance techniques. In this paper we demonstrate the experimental determination of the Néel vector in a thin film of antiferromagnetic CuMnAs9,10 which is the prominent material used in the first realization of antiferromagnetic memory chips.10 We employ a femtosecond pump-probe magneto-optical experiment based on magnetic linear dichroism. This table-top optical method is considerably more accessible than the traditionally employed large scale facility techniques like neutron diffraction11 and Xray magnetic dichroism measurements.12-14 This optical technique allows an unambiguous direct determination of the Néel vector orientation in thin antiferromagnetic films utilized in devices directly from measured data without fitting to a theoretical model
Field-driven femtosecond magnetization dynamics induced by ultrastrong coupling to THz transients
Controlling ultrafast magnetization dynamics by a femtosecond laser is
attracting interest both in fundamental science and industry because of the
potential to achieve magnetic domain switching at ever advanced speed. Here we
report experiments illustrating the ultrastrong and fully coherent light-matter
coupling of a high-field single-cycle THz transient to the magnetization vector
in a ferromagnetic thin film. We could visualize magnetization dynamics which
occur on a timescale of the THz laser cycle and two orders of magnitude faster
than the natural precession response of electrons to an external magnetic
field, given by the Larmor frequency. We show that for one particular
scattering geometry the strong coherent optical coupling can be described
within the framework of a renormalized Landau Lifshitz equation. In addition to
fundamentally new insights to ultrafast magnetization dynamics the coherent
interaction allows for retrieving the complex time-frequency magnetic
properties and points out new opportunities in data storage technology towards
significantly higher storage speed.Comment: 25 page
Vectorial Control of Magnetization by Light
Coherent light-matter interactions have recently extended their applications
to the ultrafast control of magnetization in solids. An important but
unrealized technique is the manipulation of magnetization vector motion to make
it follow an arbitrarily designed multi-dimensional trajectory. Furthermore,
for its realization, the phase and amplitude of degenerate modes need to be
steered independently. A promising method is to employ Raman-type nonlinear
optical processes induced by femtosecond laser pulses, where magnetic
oscillations are induced impulsively with a controlled initial phase and an
azimuthal angle that follows well defined selection rules determined by the
materials' symmetries. Here, we emphasize the fact that temporal variation of
the polarization angle of the laser pulses enables us to distinguish between
the two degenerate modes. A full manipulation of two-dimensional magnetic
oscillations is demonstrated in antiferromagnetic NiO by employing a pair of
polarization-twisted optical pulses. These results have lead to a new concept
of vectorial control of magnetization by light
Experimental observation of the optical spin transfer torque
The spin transfer torque is a phenomenon in which angular momentum of a spin
polarized electrical current entering a ferromagnet is transferred to the
magnetization. The effect has opened a new research field of electrically
driven magnetization dynamics in magnetic nanostructures and plays an important
role in the development of a new generation of memory devices and tunable
oscillators. Optical excitations of magnetic systems by laser pulses have been
a separate research field whose aim is to explore magnetization dynamics at
short time scales and enable ultrafast spintronic devices. We report the
experimental observation of the optical spin transfer torque, predicted
theoretically several years ago building the bridge between these two fields of
spintronics research. In a pump-and-probe optical experiment we measure
coherent spin precession in a (Ga,Mn)As ferromagnetic semiconductor excited by
circularly polarized laser pulses. During the pump pulse, the spin angular
momentum of photo-carriers generated by the absorbed light is transferred to
the collective magnetization of the ferromagnet. We interpret the observed
optical spin transfer torque and the magnetization precession it triggers on a
quantitative microscopic level. Bringing the spin transfer physics into optics
introduces a fundamentally distinct mechanism from the previously reported
thermal and non-thermal laser excitations of magnets. Bringing optics into the
field of spin transfer torques decreases by several orders of magnitude the
timescales at which these phenomena are explored and utilized.Comment: 11 pages, 4 figure
Femtosecond control of electric currents at the interfaces of metallic ferromagnetic heterostructures
The idea to utilize not only the charge but also the spin of electrons in the
operation of electronic devices has led to the development of spintronics,
causing a revolution in how information is stored and processed. A novel
advancement would be to develop ultrafast spintronics using femtosecond laser
pulses. Employing terahertz (10 Hz) emission spectroscopy, we
demonstrate optical generation of spin-polarized electric currents at the
interfaces of metallic ferromagnetic heterostructures at the femtosecond
timescale. The direction of the photocurrent is controlled by the helicity of
the circularly polarized light. These results open up new opportunities for
realizing spintronics in the unprecedented terahertz regime and provide new
insights in all-optical control of magnetism.Comment: 3 figures and 2 tables in the main tex
Ultrafast heating as a sufficient stimulus for magnetization reversal in a ferrimagnet.
The question of how, and how fast, magnetization can be reversed is a topic of great practical interest for the manipulation and storage of magnetic information. It is generally accepted that magnetization reversal should be driven by a stimulus represented by time-non-invariant vectors such as a magnetic field, spin-polarized electric current, or cross-product of two oscillating electric fields. However, until now it has been generally assumed that heating alone, not represented as a vector at all, cannot result in a deterministic reversal of magnetization, although it may assist this process. Here we show numerically and demonstrate experimentally a novel mechanism of deterministic magnetization reversal in a ferrimagnet driven by an ultrafast heating of the medium resulting from the absorption of a sub-picosecond laser pulse without the presence of a magnetic field
Phonon-driven spin-Floquet magneto-valleytronics in MoS2
Two-dimensional materials equipped with strong spin-orbit coupling can display novel electronic, spintronic, and topological properties originating from the breaking of time or inversion symmetry. A lot of interest has focused on the valley degrees of freedom that can be used to encode binary information. By performing ab initio time-dependent density functional simulation on MoS2, here we show that the spin is not only locked to the valley momenta but strongly coupled to the optical E '' phonon that lifts the lattice mirror symmetry. Once the phonon is pumped so as to break time-reversal symmetry, the resulting Floquet spectra of the phonon-dressed spins carry a net out-of-plane magnetization (approximate to 0.024 mu(B) for single-phonon quantum) even though the original system is non-magnetic. This dichroic magnetic response of the valley states is general for all 2H semiconducting transition-metal dichalcogenides and can be probed and controlled by infrared coherent laser excitation
All-optical switching in granular ferromagnets caused by magnetic circular dichroism
Magnetic recording using circularly polarised femto-second laser pulses is an emerging technology that would allow write speeds much faster than existing field driven methods. However, the mechanism that drives the magnetisation switching in ferromagnets is unclear. Recent theories suggest that the interaction of the light with the magnetised media induces an opto-magnetic field within the media, known as the inverse Faraday effect. Here we show that an alternative mechanism, driven by thermal excitation over the anisotropy energy barrier and a difference in the energy absorption depending on polarisation, can create a net magnetisation over a series of laser pulses in an ensemble of single domain grains. Only a small difference in the absorption is required to reach magnetisation levels observed experimentally and the model does not preclude the role of the inverse Faraday effect but removes the necessity that the opto-magnetic field is 10 s of Tesla in strength
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